Please use this identifier to cite or link to this item: http://hdl.handle.net/2440/113650
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Type: Journal article
Title: Size-tailored porous spheres of manganese oxides for catalytic oxidation via peroxymonosulfate activation
Author: Liu, Q.
Duan, X.
Sun, H.
Wang, Y.
Tade, M.
Wang, S.
Citation: Journal of Physical Chemistry C, 2016; 120(30):16871-16878
Publisher: American Chemical Society
Issue Date: 2016
ISSN: 1932-7447
1932-7455
Statement of
Responsibility: 
Qiaoran Liu, Xiaoguang Duan, Hongqi Sun, Yuxian Wang, Moses O. Tade, and Shaobin Wang
Abstract: Highly porous and monodisperse manganese oxides with different particle sizes were synthesized via a one-pot hydration and annealing process. Their catalytic performances were evaluated by the activation of peroxymonosulfate (PMS) to degrade phenol in aqueous solutions. The effects of sphere size (200−500 nm), calcination temperature (200−1000 °C), catalytic stability (leaching problem and reusability), reaction kinetics, and reaction temperature (25−45 °C) on the degradation efficiencies as well as the degradation mechanism were comprehensively studied. The small sized catalyst displayed the best efficiency in decomposition of phenol, and the annealing treatments would significantly improve the catalytic stability.
Description: Published: July 6, 2016
Rights: © 2016 American Chemical Society
RMID: 0030095314
DOI: 10.1021/acs.jpcc.6b05934
Grant ID: http://purl.org/au-research/grants/arc/DP150103026
Appears in Collections:Chemical Engineering publications

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