Please use this identifier to cite or link to this item: http://hdl.handle.net/2440/119442
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dc.contributor.authorWang, X.en
dc.contributor.authorVasileff, A.en
dc.contributor.authorJiao, Y.en
dc.contributor.authorZheng, Y.en
dc.contributor.authorQiao, S.en
dc.date.issued2019en
dc.identifier.citationAdvanced Materials, 2019; 31(13):1803625en
dc.identifier.issn0935-9648en
dc.identifier.issn1521-4095en
dc.identifier.urihttp://hdl.handle.net/2440/119442-
dc.description.abstractSince first being reported as possible electrocatalysts to substitute platinum for the oxygen reduction reaction (ORR), carbon-based metal-free nanomaterials have been considered a class of promising low-cost materials for clean and sustainable energy-conversion reactions. However, beyond the ORR, the development of carbon-based catalysts for other electrocatalytic reactions is still limited. More importantly, the intrinsic activity of most carbon-based metal-free catalysts is inadequate compared to their metal-based counterparts. To address this challenge, more design strategies are needed in order to improve the overall performance of carbon-based materials. Herein, using water splitting as an example, some state-of-the-art strategies in promoting carbon-based nanomaterials are summarized, including graphene, carbon nanotubes, and graphitic-carbon nitride, as highly active electrocatalysts for hydrogen evolution and oxygen evolution reactions. It is shown that by rationally tuning the electronic and/or physical structure of the carbon nanomaterials, adsorption of reaction intermediates is optimized, consequently improving the apparent electrocatalytic performance. These strategies may facilitate the development in this area and lead to the discovery of advanced carbon-based nanomaterials for various applications in energy-conversion processes.en
dc.description.statementofresponsibilityXuesi Wang, Anthony Vasileff, Yan Jiao, Yao Zheng, Shi‐Zhang Qiaoen
dc.language.isoenen
dc.publisherWiley Online Libraryen
dc.rights© 2018 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheimen
dc.subjectcarbon engineering; hydrogen evolution reactions; metal-free electrocatalysts; oxygen evolution reactions; water splittingen
dc.titleElectronic and structural engineering of carbon-based metal-free electrocatalysts for water splittingen
dc.typeJournal articleen
dc.identifier.rmid0030099124en
dc.identifier.doi10.1002/adma.201803625en
dc.relation.granthttp://purl.org/au-research/grants/arc/DE160101163en
dc.relation.granthttp://purl.org/au-research/grants/arc/DP160104866en
dc.relation.granthttp://purl.org/au-research/grants/arc/LP160100927en
dc.relation.granthttp://purl.org/au-research/grants/arc/FL170100154en
dc.relation.granthttp://purl.org/au-research/grants/arc/DP170104464en
dc.identifier.pubid440632-
pubs.library.collectionChemical Engineering publicationsen
pubs.library.teamDS10en
pubs.verification-statusVerifieden
pubs.publication-statusPublisheden
dc.identifier.orcidWang, X. [0000-0002-2477-8111]en
dc.identifier.orcidVasileff, A. [0000-0003-1945-7740]en
dc.identifier.orcidJiao, Y. [0000-0003-1329-4290]en
dc.identifier.orcidZheng, Y. [0000-0002-2411-8041]en
dc.identifier.orcidQiao, S. [0000-0002-1220-1761]en
Appears in Collections:Chemical Engineering publications

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