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https://hdl.handle.net/2440/125012
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dc.contributor.author | Tian, W. | - |
dc.contributor.author | Sun, H. | - |
dc.contributor.author | Duan, X. | - |
dc.contributor.author | Zhang, H. | - |
dc.contributor.author | Ren, Y. | - |
dc.contributor.author | Wang, S. | - |
dc.date.issued | 2019 | - |
dc.identifier.citation | Journal of Hazardous Materials, 2019; 389:121881-1-121881-9 | - |
dc.identifier.issn | 0304-3894 | - |
dc.identifier.issn | 1873-3336 | - |
dc.identifier.uri | http://hdl.handle.net/2440/125012 | - |
dc.description.abstract | The biomass, bottlebrush flower, is exploited for the preparation of functionalized porous carbons by one-pot thermal activation using NaHCO3 and dicyandiamide. An intensified cross-linking effect among the precursors boosts pore (especially mesopore) formation in the pyrolysis process, producing N-doped porous carbons (NPCs) with a large specific surface area (SSA, up to 2025 m2 g-1). The biomass-derived carbon samples turn out to be highly effective in adsorption, and catalytic activation of peroxymonosulfate for degradation of aqueous phenol and p-hydroxybenzoic acid (HBA) in single and binary systems. The effects of N content, porous structure, and trace Ni species on the adsorptive and catalytic behavior of carbon are investigated. It is found that the porous structure plays a more critical role in adsorption than surface N functionality, while the contributions of various reactive species for phenol and HBA degradation are different. | - |
dc.description.statementofresponsibility | Wenjie Tian, Hongqi Sun, Xiaoguang Duan, Huayang Zhang, Yongxiang Ren, Shaobin Wang | - |
dc.language.iso | en | - |
dc.publisher | Elsevier | - |
dc.rights | © 2019 Elsevier B.V. All rights reserved. | - |
dc.source.uri | http://dx.doi.org/10.1016/j.jhazmat.2019.121881 | - |
dc.subject | Adsorption | - |
dc.subject | Advanced oxidation processes | - |
dc.subject | Biomass | - |
dc.subject | Functionalized porous carbon | - |
dc.subject | Multicomponent system | - |
dc.title | Biomass-derived functional porous carbons for adsorption and catalytic degradation of binary micropollutants in water | - |
dc.type | Journal article | - |
dc.identifier.doi | 10.1016/j.jhazmat.2019.121881 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/DP190103548 | - |
pubs.publication-status | Published | - |
dc.identifier.orcid | Tian, W. [0000-0002-9896-1154] | - |
dc.identifier.orcid | Duan, X. [0000-0001-9635-5807] | - |
dc.identifier.orcid | Wang, S. [0000-0002-1751-9162] | - |
Appears in Collections: | Aurora harvest 4 Chemical Engineering publications |
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