Please use this identifier to cite or link to this item: http://hdl.handle.net/2440/128188
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dc.contributor.authorTang, C.en
dc.contributor.authorZhang, Q.en
dc.date.issued2017en
dc.identifier.citationAdvanced Materials, 2017; 29(13):1604103-1-1604103-9en
dc.identifier.issn0935-9648en
dc.identifier.issn1521-4095en
dc.identifier.urihttp://hdl.handle.net/2440/128188-
dc.description.abstractThe oxygen reduction reaction (ORR) is the cornerstone of various sustainable energy‐conversion technologies. Metal‐free nanocarbon electrocatalysts with competitive activity, enhanced durability, and satisfactory cost, have been proposed as the most promising substitute for precious‐metal catalysts. However, their further development is still primarily based on trial‐and‐error approaches due to the controversial knowledge of critical active sites and mechanisms. Herein, the activity origins of nanocarbon‐based ORR electro­catalysts are comprehensively reviewed and correlated, considering the dopants, edges, and defects. Analogously, they can effectively modify the charge/spin distribution on the sp²‐conjugated carbon matrix, leading to optimized intermediate chemisorption and facilitated electron transfer. Specific doping at defective edges is expected to render practical applications for metal‐free nanocarbon electrocatalysts.en
dc.description.statementofresponsibilityCheng Tang and Qiang Zhangen
dc.language.isoenen
dc.publisherWileyen
dc.rights© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheimen
dc.subjectDefects; doping; edge effect; nanocarbon catalysis; oxygen reductionen
dc.titleNanocarbon for oxygen reduction electrocatalysis: dopants, edges, and defectsen
dc.typeJournal articleen
dc.identifier.rmid1000020499en
dc.identifier.doi10.1002/adma.201604103en
dc.identifier.pubid531558-
pubs.library.collectionChemical Engineering publicationsen
pubs.library.teamDS14en
pubs.verification-statusVerifieden
pubs.publication-statusPublisheden
dc.identifier.orcidTang, C. [0000-0002-5167-1192]en
Appears in Collections:Chemical Engineering publications

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