Please use this identifier to cite or link to this item: http://hdl.handle.net/2440/129270
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Type: Journal article
Title: Destabilizing alkaline water by 3d-metal (oxy)(hydr)oxides for improved hydrogen evolution
Author: You, B.
Qiao, S.
Citation: Chemistry, 2021; 27(2):553-564
Publisher: Wiley
Issue Date: 2021
ISSN: 0947-6539
1521-3765
Statement of
Responsibility: 
Bo You, Shi Zhang Qiao
Abstract: Alkaline water electrolysis enables the use of nonprecious metal-based catalysts and therefore holds great promise for large-scale generation of renewable hydrogen fuel, especially when driven by renewable energy sources, such solar and wind. However, the sluggish kinetics of water adsorption and dissociation steps in alkaline hydrogen evolution reaction (HER) lower its energy conversion efficiency. Recent achievements have proved that 3d -metal (oxy)(hydr)oxides can accelerate these two kinetic processes and thereby improve the activity of diverse HER electrocatalysts from experimental and theoretical points of view. Moreover, a positive role of strong coupling between HER catalysts and 3d -metal (oxy)(hydr)oxides has been discovered recently. In this minireview we provide a compendious introduction to recent progress, including experiments and theory. Remarks on challenges and perspectives in this rapidly developing field are also provided.
Keywords: alkaline medium; electrocatalysis; hydrogen evolution; interface engineering; water dissociation
Description: Version of record online: October 13, 2020
Rights: © 2020 Wiley‐VCH GmbH
RMID: 1000024392
DOI: 10.1002/chem.202002503
Grant ID: http://purl.org/au-research/grants/arc/FL170100154
http://purl.org/au-research/grants/arc/DP160104866
http://purl.org/au-research/grants/arc/LP160100927
Appears in Collections:Physics publications

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