Biomimetic total synthesis of the rubiginosin meroterpenoids
Date
2021
Authors
Burchill, L.
Day, A.J.
Yahiaoui, O.
George, J.H.
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Journal article
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Organic Letters, 2021; 23(2):578-582
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Laura Burchill, Aaron J. Day, Oussama Yahiaoui, and Jonathan H. George
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Abstract
Total synthesis of the <i>Rhododendron</i> meroterpenoids rubiginosins A and G, which both contain unusual 6-6-6-4 ring systems, has been achieved using a bioinspired cascade approach. Stepwise synthesis of these natural products, and the related 6-6-5-4 meroterpenoids fastinoid B and rhodonoid B, from naturally occurring chromene precursors is also reported.
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© 2020 American Chemical Society