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https://hdl.handle.net/2440/85361
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Type: | Journal article |
Title: | Rotational study of carbon monoxide solvated with helium atoms |
Author: | Surin, L. Potapov, A. Dumesh, B. Schlemmer, S. Xu, Y. Raston, P. Jager, W. |
Citation: | Physical Review Letters, 2008; 101(23):233401-1-233401-4 |
Publisher: | American Physical Society |
Issue Date: | 2008 |
ISSN: | 0031-9007 1079-7114 |
Statement of Responsibility: | L. A. Surin, A. V. Potapov, B. S. Dumesh, S. Schlemmer, Y. Xu, P. L. Raston, and W. Jäger |
Abstract: | High resolution microwave and millimeter-wave spectra of HeN-CO clusters with N up to 10, produced in a molecular expansion, were observed. Two series of J = 1-0 transitions were detected, which correspond to the a-type and b-type J = 1-0 transitions of He1-CO. The B rotational constant initially decreases with N and reaches a minimum at N = 3. Its subsequent rise indicates the transition from a molecular complex to a quantum solvated system already for N = 4. For N > or =6, the B value becomes larger than that of He1-CO, indicating an almost free rotation of CO within the helium environment. |
Rights: | © 2008 The American Physical Society |
DOI: | 10.1103/PhysRevLett.101.233401 |
Published version: | http://dx.doi.org/10.1103/physrevlett.101.233401 |
Appears in Collections: | Aurora harvest 2 Physics publications |
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