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https://hdl.handle.net/2440/111677
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dc.contributor.author | Batmunkh, M. | - |
dc.contributor.author | Shrestha, A. | - |
dc.contributor.author | Bat-Erdene, M. | - |
dc.contributor.author | Nine, M. | - |
dc.contributor.author | Shearer, C. | - |
dc.contributor.author | Gibson, C. | - |
dc.contributor.author | Slattery, A. | - |
dc.contributor.author | Tawfik, S. | - |
dc.contributor.author | Ford, M. | - |
dc.contributor.author | Dai, S. | - |
dc.contributor.author | Qiao, S. | - |
dc.contributor.author | Shapter, J. | - |
dc.date.issued | 2018 | - |
dc.identifier.citation | Angewandte Chemie International Edition, 2018; 57(10):2644-2647 | - |
dc.identifier.issn | 1433-7851 | - |
dc.identifier.issn | 1521-3773 | - |
dc.identifier.uri | http://hdl.handle.net/2440/111677 | - |
dc.description.abstract | Research into efficient synthesis, fundamental properties, and potential applications of phosphorene is currently the subject of intense investigation. Herein, solution-processed phosphorene or few-layer black phosphorus (FL-BP) sheets are prepared using a microwave exfoliation method and used in photoelectrochemical cells. Based on experimental and theoretical (DFT) studies, the FL-BP sheets are found to act as catalytically active sites and show excellent electrocatalytic activity for triiodide reduction in dye-sensitized solar cells. Importantly, the device fabricated based on the newly designed cobalt sulfide (CoSx ) decorated nitrogen and sulfur co-doped carbon nanotube heteroelectrocatalyst coated with FL-BP (FL-BP@N,S-doped CNTs-CoSx ) displayed an impressive photovoltaic efficiency of 8.31 %, outperforming expensive platinum based cells. This work paves the way for using phosphorene-based electrocatalysts for next-generation energy-storage systems. | - |
dc.description.statementofresponsibility | Munkhbayar Batmunkh, Aabhash Shrestha, Munkhjargal Bat-Erdene, Md Julker Nine, Cameron J. Shearer, Christopher T. Gibson, Ashley D. Slattery, Sherif Abdulkader Tawfik, Michael J. Ford, Sheng Dai, Shizhang Qiao, and Joseph G. Shapter | - |
dc.language.iso | en | - |
dc.publisher | Wiley | - |
dc.rights | © 2018 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim | - |
dc.source.uri | http://dx.doi.org/10.1002/anie.201712280 | - |
dc.subject | 2D materials; black phosphorus; electrocatalysis; photochemistry; solar cells | - |
dc.title | Electrocatalytic activity of a 2D phosphorene-based heteroelectrocatalyst for photoelectrochemical cells | - |
dc.type | Journal article | - |
dc.identifier.doi | 10.1002/anie.201712280 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/DP150101354 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/DP160101301 | - |
pubs.publication-status | Published | - |
dc.identifier.orcid | Nine, M. [0000-0002-5740-8627] | - |
dc.identifier.orcid | Shearer, C. [0000-0002-8192-3696] | - |
dc.identifier.orcid | Slattery, A. [0000-0003-4023-3506] | - |
dc.identifier.orcid | Qiao, S. [0000-0002-1220-1761] [0000-0002-4568-8422] | - |
Appears in Collections: | Aurora harvest 3 Chemical Engineering publications |
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