Please use this identifier to cite or link to this item: https://hdl.handle.net/2440/137318
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Type: Journal article
Title: Efficient photothermal deicing employing superhydrophobic plasmonic MXene composites
Author: Wang, J.
Li, P.
Yu, P.
Leydecker, T.
Bayer, I.S.
Losic, D.
Neogi, A.
Wang, Z.
Citation: Advanced Composites and Hybrid Materials, 2022; 5(4):3035-3044
Publisher: Springer Nature
Issue Date: 2022
ISSN: 2522-0128
2522-0136
Statement of
Responsibility: 
Jiaying Wang, Peihang Li, Peng Yu, Tim Leydecker, Ilker S. Bayer, Dusan Losic, Arup Neogi, Zhiming Wang
Abstract: Deicing and anti-icing on the surface, such as train tracks, highways, airports, aircraft, cars, ships, wind turbines, and outdoor cables, represent a significant challenge. Many different chemical compounds and coatings were explored and used to address these problems, but some limitations remain. The anti-icing ability under low temperature and high humidity conditions, the low deicing efficiency, and the complex preparation method, etc., restrict the application and development of deicing materials. This paper presents a simple and efficient solution based on new plasmonic photothermal superhydrophobic composite coatings. A hybrid MXene@Au-waterborne polyurethane (MXene@Au-WPU) coating is specifically designed to realize a significant temperature rise due to the high absorption and rapid heat transfer of the plasmonic MXene@Au in the entire coating. To achieve superhydrophobicity, chemically modifed SiO2 nanoparticles were deposited on the surface of the MXene@Au-WPU layer to obtain a fSiO2/MXene@Au-WPU(fuoroalkyl silanes-SiO2/MXene@Au-WPU) superhydrophobic photothermal coating featuring a contact angle of 153°. The composite coating was demonstrated to be adequate for anti-icing and deicing applications, with an ultra-long anti-icing time of 1053 s under low temperature and high humidity conditions (−20 °C, relative humidity 68%). Compared to previous work, the coating also achieved a super high photothermal deicing efficiency of 73.1%. The result presented in the article furthermore demonstrates resistance to corrosive liquids with pH ranging from 1 to 13. A combination of the anti-icing, corrosion-resistance, and facile implementation features of this multifunctional coating enhances its high potential for implementation in various surface technologies.
Keywords: Photothermal deicing; Superhydrophobic; MXene; Plasmonic; Composite coating
Rights: © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022
DOI: 10.1007/s42114-022-00549-5
Grant ID: http://purl.org/au-research/grants/arc/IH150100003
Appears in Collections:Chemical Engineering publications

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