Modelling of PFAS-surface interactions: effect of surface charge and solution ions

Date

2023

Authors

Sleep, J.A.
Miklavcic, S.J.
Juhasz, A.L.

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Journal article

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Chemosphere, 2023; 319(137910):1-10

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Abstract

Per-and poly-fluoroalkyl substances (PFAS) are a class of substances of increasing concern as environmental contaminants. The interactions between PFAS and surfaces play an important role in PFAS transport and remediation. Previous studies have found PFAS adsorption to be dependent upon properties including pH, organic matter and particle size, along with PFAS functional group and carbon chain length. It is hypothesised that a theoretical examination of PFAS-surface interactions, via Monte Carlo molecular simulation, would show differences resulting from changes in surface charge, H⁺, OH⁻, Ca²⁺ concentrations and PFAS carbon chain length. Monte Carlo molecular simulations of perfluorooctane and perfluorobutane sulfonic acids interacting with a graphite surface in an aqueous medium were performed. Variations in surface charge, H⁺, OH⁻ and Ca²⁺ concentrations were made. The distance-dependent density of molecules from the surface was analysed as a proxy for PFAS adsorption to the surface. Simulation results showed differences in surface behaviour that depended on surface charge, H⁺, OH⁻ and Ca²⁺ concentrations, along with carbon chain length, with surface charge playing the most prominent role in controlling PFAS adsorption. For negatively charged surfaces, adsorption due to divalent cation bridging was observed in Ca²⁺ solutions. Modelling, such as in this study, of the thermodynamic equilibrium behaviour of low concentrations of molecules, in scenarios where both adsorption and mobility of PFAS occur, can aid in the design and testing of sorptive surfaces for amendment-based PFAS remediation.

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Data source: Supplementary data, https://doi.org/10.1016/j.chemosphere.2023.137910

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Copyright 2023 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/bync-nd/4.0/)

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