Arsenic in marine organisms: new species and new analytical approaches

Date

2012

Authors

Maher, W.A.
Foster, S.
Krikowa, F.
Duncan, E.
Raber, G.
Francesconi, K.A.

Editors

Ng, J.C.

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Conference paper

Citation

Understanding the geological and medical interface of arsenic: As 2012, 2012 / Ng, J.C. (ed./s), pp.363-366

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4th International Congress on Arsenic in the Environment - Understanding the Geological and Medical Interface (As) (22 Jul 2012 - 27 Jul 2012 : Cairns, Australia)

Abstract

Recently two new classes of arsenic species have been identified in marine organisms; thio-arsenic species where the oxygen bonded to arsenic is replaced by a sulphur group and two types of arsenic-lipids, arsenic hydrocarbons and arsenic phospholipids. Here we describe the common species found in marine and HPLC-ICPMS analytical approaches to measure these species. Thio-arsenic species can be separated using C18 reverse phase chromatography with elution with aqueous phosphate buffer. Arsenic-lipids can be separated by C8 reverse phase chromatography with gradient elution comprising acetic acid and methanol with gradient elution conditions: 0-25 min, 50%-95% methanol; 25-40 min, 95% methanol. Using gradients, the introduction of methanol directly into the ICPMS spray chamber is required to compensate for the variable amounts of carbon in the mobile phase entering the ICPMS.

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Copyright 2012 Taylor and Francis Group

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