Heteroatom-doped graphene-based materials for energy-relevant electrocatalytic processes
| dc.contributor.author | Duan, J. | |
| dc.contributor.author | Chen, S. | |
| dc.contributor.author | Jaroniec, M. | |
| dc.contributor.author | Qiao, S. | |
| dc.date.issued | 2015 | |
| dc.description.abstract | To address aggravating energy and environment issues, inexpensive, highly active, and durable electrocatalysts as noble metal substitutes both at the anode and cathode are being actively pursued. Among them, heteroatom-doped graphene-based materials show extraordinary electrocatalytic performance, some even close to or outperforming the state-of-the-art noble metals, such as Pt- and IrO₂- based materials. This review provides a concise appraisal on graphene doping methods, possible doping configurations and their unique electrochemical properties, including single and double doping with N, B, S, and P. In addition, heteroatom-doped graphene-based materials are reviewed as electrocatalysts for oxygen reduction, hydrogen evolution, and oxygen evolution reactions in terms of their electrocatalytic mechanisms and performance. Significantly, three-dimensional heteroatom-doped graphene structures have been discussed, and those especially can be directly utilized as catalyst electrodes without extra binders and supports. | |
| dc.description.statementofresponsibility | Jingjing Duan, Sheng Chen, Mietek Jaroniec, and Shi Zhang Qiao | |
| dc.identifier.citation | ACS Catalysis, 2015; 5(9):5207-5234 | |
| dc.identifier.doi | 10.1021/acscatal.5b00991 | |
| dc.identifier.issn | 2155-5435 | |
| dc.identifier.issn | 2155-5435 | |
| dc.identifier.orcid | Qiao, S. [0000-0002-1220-1761] [0000-0002-4568-8422] | |
| dc.identifier.uri | http://hdl.handle.net/2440/100885 | |
| dc.language.iso | en | |
| dc.publisher | American Chemical Society | |
| dc.relation.grant | http://purl.org/au-research/grants/arc/DP130104459 | |
| dc.relation.grant | http://purl.org/au-research/grants/arc/DP140104062 | |
| dc.rights | © 2015 American Chemical Society | |
| dc.source.uri | https://doi.org/10.1021/acscatal.5b00991 | |
| dc.subject | Heteroatom-doped graphene; nonnoble electrocatalysts; oxygen reduction reaction; hydrogen evolution reaction; oxygen evolution reaction | |
| dc.title | Heteroatom-doped graphene-based materials for energy-relevant electrocatalytic processes | |
| dc.type | Journal article | |
| pubs.publication-status | Published |