Titanate-silica mesostructured nanocables: synthesis, structural analysis and biomedical applications

Date

2010

Authors

Su, Y.
Qiao, S.
Yang, H.
Yang, C.
Jin, Y.
Stahr, F.
Sheng, J.
Cheng, L.
Ling, C.
Lu, G.

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Journal article

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Nanotechnology, 2010; 21(6):online-

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Yonghua Su, Shizhang Qiao, Huagui Yang, ChenYang, Yonggang Jin, Frances Stahr, Jiayu Sheng, Lina Cheng, Changquan Ling, and Gao Qing Lu

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Abstract

1D hierarchical composite mesostructures of titanate and silica were synthesized via an interfacial surfactant templating approach. Such mesostructures have complex core–shell architectures consisting of single-crystalline H₂Ti₃O₇ nanobelts inside the ordered mesoporous SiO₂ shell, which are nontoxic and highly biocompatible. The overall diameter of as-prepared 1D hierarchical composite mesostructures is only approx. 34.2 nm with a length over 500 nm on average. A model to explain the formation mechanism of these mesostructures has been proposed; the negatively charged surface of H₂Ti₃O₇ nanobelts controls the formation of the octadecyltrimethylammonium bromide (C₁₈TAB) bilayer, which in turn regulates the cooperative self-assembly of silica and C₁₈TAB complex micelles on the interface to produce a mesoporous silica shell. More importantly, the application of synthesized mesostructured nanocables as anticancer drug reservoirs has also been explored, which indicates that the membranes containing these mesoporous nanocables have a great potential to be used as transdermal drug delivery systems.

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© 2010 IOP Publishing Ltd

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