Dynamic Active Sites in Electrocatalysis

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dc.contributor.authorNing, M.
dc.contributor.authorWang, S.
dc.contributor.authorWan, J.
dc.contributor.authorXi, Z.
dc.contributor.authorChen, Q.
dc.contributor.authorSun, Y.
dc.contributor.authorLi, H.
dc.contributor.authorMa, T.
dc.contributor.authorJin, H.
dc.contributor.authorJin, H.
dc.date.issued2024
dc.descriptionVersion of record online: October 31, 2024
dc.description.abstractIn-depth understanding of the real-time behaviors of active sites during electrocatalysis is essential for the advancement of sustainable energy conversion. Recently, the concept of dynamic active sites has been recognized as a potent approach for creating self-adaptive electrocatalysts that can address a variety of electrocatalytic reactions, outperforming traditional electrocatalysts with static active sites. Nonetheless, the comprehension of the underlying principles that guide the engineering of dynamic active sites is presently insufficient. In this review, we systematically analyze the fundamentals of dynamic active sites for electrocatalysis and consider important future directions for this emerging field. We reveal that dynamic behaviors and reversibility are two crucial factors that influence electrocatalytic performance. By reviewing recent advances in dynamic active sites, we conclude that implementing dynamic electrocatalysis through variable reaction environments, correlating the model of dynamic evolution with catalytic properties, and developing localized and ultrafast in situ/operando techniques are keys to designing high-performance dynamic electrocatalysts. This review paves the way to the development of the next-generation electrocatalyst and the universal theory for both dynamic and static active sites.
dc.description.statementofresponsibilityMinghui Ning, Sangni Wang, Jun Wan, Zichao Xi, Qiao Chen, Yuanmiao Sun, Hui Li, Tianyi Ma, and Huanyu Jin
dc.identifier.citationAngewandte Chemie International Edition, 2024; 63(50):e202415794-1-e202415794-17
dc.identifier.doi10.1002/anie.202415794
dc.identifier.issn1433-7851
dc.identifier.issn1521-3773
dc.identifier.orcidJin, H. [0000-0002-1950-2364]
dc.identifier.urihttps://hdl.handle.net/2440/144251
dc.language.isoen
dc.publisherWiley
dc.relation.granthttp://purl.org/au-research/grants/arc/FT210100298
dc.relation.granthttp://purl.org/au-research/grants/arc/DP220100603
dc.relation.granthttp://purl.org/au-research/grants/arc/LP210200504
dc.relation.granthttp://purl.org/au-research/grants/arc/LP220100088
dc.relation.granthttp://purl.org/au-research/grants/arc/LP230200897
dc.relation.granthttp://purl.org/au-research/grants/arc/IH240100009
dc.rights© 2024 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
dc.source.urihttps://doi.org/10.1002/anie.202415794
dc.subjectdynamic active sites
dc.subjectdynamic reconstruction
dc.subjectelectrocatalysis
dc.subjectin situ/operando characterization
dc.subjectstructure–activity correlations
dc.titleDynamic Active Sites in Electrocatalysis
dc.typeJournal article
pubs.publication-statusPublished

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