Microenvironment Engineering of Heterogeneous Catalysts for Liquid-Phase Environmental Catalysis

Simple item page
dc.contributor.authorZhu, Z.-S.
dc.contributor.authorZhong, S.
dc.contributor.authorCheng, C.
dc.contributor.authorZhou, H.
dc.contributor.authorSun, H.
dc.contributor.authorDuan, X.
dc.contributor.authorWang, S.
dc.date.issued2024
dc.description.abstractEnvironmental catalysis has emerged as a scientific frontier in mitigating water pollution and advancing circular chemistry and reaction microenvironment significantly influences the catalytic performance and efficiency. This review delves into microenvironment engineering within liquid-phase environmental catalysis, categorizing microenvironments into four scales: atom/molecule-level modulation, nano/microscale-confined structures, interface and surface regulation, and external field effects. Each category is analyzed for its unique characteristics and merits, emphasizing its potential to significantly enhance catalytic efficiency and selectivity. Following this overview, we introduced recent advancements in advanced material and system design to promote liquid-phase environmental catalysis (e.g., water purification, transformation to value-added products, and green synthesis), leveraging state-of-the-art microenvironment engineering technologies. These discussions showcase microenvironment engineering was applied in different reactions to fine-tune catalytic regimes and improve the efficiency from both thermodynamics and kinetics perspectives. Lastly, we discussed the challenges and future directions in microenvironment engineering. This review underscores the potential of microenvironment engineering in intelligent materials and system design to drive the development of more effective and sustainable catalytic solutions to environmental decontamination.
dc.description.statementofresponsibilityZhong-Shuai Zhu, Shuang Zhong, Cheng Cheng, Hongyu Zhou, Hongqi Sun, Xiaoguang Duan, Shaobin Wang
dc.identifier.citationChemical Reviews, 2024; 124(20):11348-11434
dc.identifier.doi10.1021/acs.chemrev.4c00276
dc.identifier.issn0009-2665
dc.identifier.issn1520-6890
dc.identifier.orcidZhu, Z.-S. [0000-0001-8821-2136]
dc.identifier.orcidZhong, S. [0000-0001-6103-5125]
dc.identifier.orcidZhou, H. [0000-0003-1117-1422]
dc.identifier.orcidDuan, X. [0000-0001-9635-5807]
dc.identifier.orcidWang, S. [0000-0002-1751-9162]
dc.identifier.urihttps://hdl.handle.net/2440/143917
dc.language.isoen
dc.publisherAmerican Chemical Society (ACS)
dc.relation.granthttp://purl.org/au-research/grants/arc/FT230100526
dc.relation.granthttp://purl.org/au-research/grants/arc/FL230100178
dc.relation.granthttp://purl.org/au-research/grants/arc/DP230102406
dc.rights© 2024 American Chemical Society
dc.source.urihttp://dx.doi.org/10.1021/acs.chemrev.4c00276
dc.subjectAdsorption; Catalysts; Electronic structure; Metals; Selectivity
dc.titleMicroenvironment Engineering of Heterogeneous Catalysts for Liquid-Phase Environmental Catalysis
dc.typeJournal article
pubs.publication-statusPublished

Files

Collections

Research Outputs